Since the layers spotify update, it is no longer possible to long press a track and remove the download. I can unlike the song but the download remains, some songs I only want to listen to when I'm streaming and I don't want them on my device.
I want to download specific songs from an album or remove specific songs from an already downloaded album.
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I have IOS so this may not work the same for you but I ended up added the songs I wanted downloaded to a playlist that I have downloaded and then flipping the whole album from undownloaded to downloaded and then back to undownloaded. Everything after that was in a downloaded playlist somewhere. I had to go searching for some of them because I didn’t realize I had them in a downloaded playlist and thought they should have been undownloaded. Hope this helps!